Teacher

Associate Professor of Chemical Engineering

Division of Nuclear Chemical Engineering

yegang@mail.tsinghua.edu.cn

(+ 86 10) 8979-6063


Education background

Ph.D.,  Tsinghua University, Material Science and Engineering, 2010
B.S.,  Tsinghua University, Polymer Science and Engineering, 2005

 

Experience

10/2013-present,  Associate Professor, Division of Nuclear Chemical Engineering, INET
07/2010-10/2013,  Assistant Professor, Division of Nuclear Chemical Engineering, INET

 

Social service

Teaching

Adsorption  Science and Technology (in preparation)

Journal Reviewer

Journal  of American Chemical Society
Advanced  Materials
Advanced  Functional Materials
Environmental  Science & Technology
Macromolecules
ACS  Macro Letters
Journal  of Materials Chemistry A
ACS  Applied Materials & Interfaces
Applied  Catalysis B
Carbon
Small

Service to Professional Associations

Environmental  Radiochemistry Committee, Nuclear chemistry and Radiochemistry Branch, CNS,  academic board
Nuclear  Chemical Engineering Committee, CNS, academic board
American  Chemical Society, member

 

Areas of Research Interests/ Research Projects

Dr. Ye’s research focuses on the task-specific development of sorbent materials for  environmental applications such as radionuclides separation, heavy metal  remediation, etc. His major interest lies in exploiting the  state-of-the-art strategies, based on polymer chemistry and biomimetic materials  science, for developing advanced sorbents while tuning their hierarchical  structures. Bearing the goal to contribute adaptable methodologies and valuable  insights to the research area of sorbent materials, over the past ten years, he  has established a series of methods for controlled architecture and surface  engineering of varieties of sorbents, as well as systematical protocols to study  their adsorption behaviors and complexation mechanisms.

Sorbents Synthesis: Surface Engineering and Structure Tuning

A critical challenge to develop high-performance sorbents for radionuclides  separation lies in the effective creation of functional moieties on the surfaces  while optimizing their binding ability. Dr. Ye  has been working on surface engineering and structural tuning of sorbents for  years. Novel strategies such as mussel-inspired polydopamine chemistry,  metal-polyphenol interaction, and photo-regulated living radical polymerization  have been exploited for the synthesis of a series of potential sorbents, showing  effective adsorption toward corresponding radioactive metal ions.

Uranium Extraction from Seawater

Developing  facile and robust technologies for effective separation of uranium from seawater  is of great significance for resource sustainability. Currently, Dr. Ye is  dedicated to the development of uranium sorbent, including  amidoxime-functionalized polymers, metal-organic frameworks (MOFs),  covalent-organic frameworks (COFs), etc., for uranium enrichment.  Except for addressing fundamental issues, Dr. Ye is also making efforts to merge  the gap between scientific principles and practical applications.

 

Research Status

2020-2022, National  Natural Science Foundation of China
Adsorption  materials of radionuclides
The  project aims to develop new synthetic strategies by taking advantage of  photo-regulated living radical polymerization techniques and the bio-inspired  metal-polyphenol interaction to prepare new functional polymer sorbents.  Meanwhile, based on the fundamental theory of polymer solutions, an in-depth  study will be carried out to clarify the influences of factors like conformation  of chain segments and coordination environment on the adsorption ability of  polymer sorbents.

2020-2022, China  National Nuclear Corporation
New  diblock copolymer sorbents for   uranium extraction from seawater:  simulation-assisted design and precise   synthesis
The  project focuses on the development of high-performance polymer sorbents for  uranium extraction from seawater, highlighting the rational design of polymer  structure with the aid of computer simulation and the precise architecture of  the target polymer structure using controlled/living radical polymerization  methods.

2018-2021,State  Administration for Science, Technology and Industry for National  Defense
Partitioning  of high-level liquid waste   (HLLW) in spent nuclear fuel reprocessing  (Sub-project III: Separation of   strontium-90 and cesium-137 from  HLLW)
The  sub-project aims to synthesize effective and selective extractants of  strontium-90 and cesium-137 while developing a solvent extraction process to  achieve efficient separation of the two fission products from HLLW.

 

Honors And Awards

National  Natural Science Fund for Excellent Young Scholar, National Natural Science  Foundation of China (NSFC)
Young  Scholar of Distinction, Tsinghua University
Metallurgical  Dean’s Award, Metallurgical Society of National University
Excellent  Doctoral Dissertation, Tsinghua University
Excellent  Graduate, Tsinghua University
National  Scholarship (1st Prize), Ministry of Education of the People’s  Republic of China

 

Academic Achievement

Publications

Zhang,  L.; Pu, N.; Yu, B.; Ye,  G.*; Chen, J.; Xu, S.; Ma, S*. Skeleton Engineering of  Homocoupled Conjugated Microporous Polymers for Highly Efficient Uranium Capture  via Synergistic Coordination. ACS Appl. Mater. Inter. 2020, 12, 3688-3696.
Jiang,  J.; Ye,  G.*; Lorandi, F.; Liu, Z.; Liu, Y.; Hu, T.; Chen, J.*; Lu, Y.;  Matyjaszewski, K.* Localized Surface Plasmon Resonance Meets Controlled/Living  Radical Polymerization: An Adaptable Strategy for Broadband Light-Regulated  Macromolecular Synthesis. Angewandte Chemie International Edition 2019, 58, 12096-12101.
Jiang,  J.; Ye,  G.*; Wang, Z.; Lu, Y.; Chen, J.*; Matyjaszewski, K.*  Heteroatom-Doped Carbon Dots (CDs) as a Class of Metal-Free Photocatalysts for  PET-RAFT Polymerization under Visible Light and Sunlight. Angew. Chem. Int.  Edit. 2018, 57, 12037-12042.
Zeng,  Z.; Wen, M.; Yu, B.; Ye,  G.*; Huo, X.; Lu, Y.; Chen, J.* Polydopamine Induced in-Situ  Formation of Metallic Nanoparticles in Confined Microchannels of Porous Membrane  as Flexible Catalytic Reactor. ACS Appl. Mater. Inter. 2018, 10, 14735-14743.
Yu,  B.; Ye,  G.*; Zeng, Z.; Zhang, L.; Chen, J.*; Ma, S.* Mussel-inspired  polydopamine chemistry to modulate template synthesis of 1D metal–organic framework superstructures. J. Mater. Chem. A 2018, 6, 21567-21576.
Yang,  Y.; Liu, X.; Ye,  G.*; Zhu, S.; Wang, Z.; Huo, X.; Matyjaszewski, K.*; Lu, Y.;  Chen, J. Metal-Free Photoinduced Electron Transfer-Atom Transfer Radical  Polymerization Integrated with Bioinspired Polydopamine Chemistry as a Green  Strategy for Surface Engineering of Magnetic Nanoparticles. ACS Appl. Mater.  Inter. 2017, 9, 13637-13646.
Wu, F.;  Pu, N.; Ye,  G.*; Sun, T.; Wang, Z.; Song, Y.; Wang, W.; Huo, X.; Lu, Y.;  Chen, J. * Performance and Mechanism of Uranium Adsorption from Seawater to  Poly(dopamine)-Inspired Sorbents. Environ. Sci. Technol. 2017, 51, 4606-4614.
Zeng,  Z.; Wen, M.; Ye,  G.*; Huo, X.; Wu, F.; Wang, Z.; Yan, J.; Matyjaszewski, K. *;  Lu, Y.; Chen, J. Controlled Architecture of Hybrid Polymer Nanocapsules with  Tunable Morphologies by Manipulating Surface-Initiated ARGET ATRP from  Hydrothermally Modified Polydopamine. Chem. Mater. 2017, 29, 10212-10219.
Song,  Y.; Ye,  G.*; Lu, Y.; Chen, J.; Wang, J. *; Matyjaszewski, K. *  Surface-Initiated ARGET ATRP of Poly(Glycidyl Methacrylate) from Carbon  Nanotubes via Bioinspired Catechol Chemistry for Efficient Adsorption of Uranium  Ions. ACS Macro Lett. 2016, 5,  382-386.
Yang,  Y.; Wang, J.; Wu, F.; Ye,  G.*; Yi, R.; Lu, Y.; Chen, J. * Surface-initiated SET-LRP  mediated by mussel-inspired polydopamine chemistry for controlled building of  novel core-shell magnetic nanoparticles for highly-efficient uranium enrichment.  Polym. Chem. 2016, 7, 2427-2435.
Song,  Y.; Ye,  G.*; Wu, F.; Wang, Z.; Liu, S.; Kopec, M.; Wang, Z.; Chen, J.;  Wang, J. *; Matyjaszewski, K. * Bioinspired Polydopamine (PDA) Chemistry Meets  Ordered Mesoporous Carbons (OMCs): A Benign Surface Modification Strategy for  Versatile Functionalization. Chem. Mater. 2016,  28, 5013-5021.
Song,  Y.; Ye,  G.*; Wang, Z.; Kopec, M.; Xie, G.; Yuan, R.; Chen, J.;  Kowalewski, T.; Wang, J.; Matyjaszewski, K. * Controlled Preparation of  Well-Defined Mesoporous Carbon/Polymer Hybrids via Surface-Initiated ICAR ATRP  with a High Dilution Strategy Assisted by Facile Polydopamine Chemistry.  Macromolecules 2016, 49,  8943-8950.
Ye,  G.*; Lee,  J.; Perreault, F.; Elimelech, M. * Controlled Architecture of Dual-Functional  Block Copolymer Brushes on Thin-Film Composite Membranes for Integrated  "Defending" and "Attacking" Strategies against Biofouling. ACS Appl. Mater.  Inter. 2015, 7, 23069-23079.
Yi, R.;  Ye,  G.*; Pan, D.; Wu, F.; Wen, M.; Chen, J. * Novel core-shell  structured superparamagnetic microspheres decorated with macrocyclic host  molecules for specific recognition and magnetic removal of Pb(II). J. Mater.  Chem. A 2014, 2, 6840-6846.
Zhang,  W.; He, X.; Ye,  G.*; Yi, R.; Chen, J. * Americium(III) Capture Using Phosphonic  Acid-Functionalized Silicas with Different Mesoporous Morphologies: Adsorption  Behavior Study and Mechanism Investigation by EXAFS/XPS. Environ. Sci.  Technol. 2014, 48, 6874-6881.
Zhang,  W.; Ye,  G.*; Chen, J. * Novel mesoporous silicas bearing phosphine oxide  ligands with different alkyl chains for the binding of uranium in strong  HNO3 media.  J. Mater. Chem. A 2013, 1,  12706-12709

Patents

Zeng  Z., Yu B., Ye G., et al. Fabrication of catalytic  membrane reactor using track-etched membrane. CN108144559A
Yu B.,  Zeng Z., Ye G., et al. A method for modification of  membrane with cylindrical pore channels. CN108211800A
Wang  W., Paziliya J., Ye G., et al. Preparation of crown  ether decorated glass fiber. CN107115846A
Liu Y.,  Ye G., Chen J. et al. Preparation of crown ether  functionalized SBA-15 ordered mesoporous silicas. CN106311153A
Liu Y.,  Ye G., Chen J. et al. Application of crown ether  decorated SBA-15 ordered mesoporous silicas. CN106268653A
Ye  G., Liu F., Liu Y., et al. Synthesis of a class of  sorbent for lithium separation. CN106179273A
Chen  J., Wu F., Ye G. Preparation of a magnetic sorbent for  palladium recovery from nitric acid media. CN105771904A
Chen  J., Wu F., Ye G. Preparation and application of a class of  modified silica-based sorbent. CN105617979A
Wu F.,  Ye G., Chen J., et al. A class of magnetic biomimetic  sorbent for treatment of uranium-containing wastewater. CN105413659A
Zhang  W., Ye G., Chen J., et al. Synthesis of a kind of  hydroxyl-containing phosphine oxide silane coupling agent.  CN103275124A
Ye  G., Leng Y., Bai F., et al. Preparation of a new kind of  calixcrown decorated silica-based sorbent, CN103055816A
Ye  G., Bai F., Wei, J., et al. Crown ether grafted silica  resin synthesized by co-condensation polymerization,  CN102875812A
Ye  G., Bai F., Wei, J., et al. Lead removal by using  single-armed cycloaliphatic crown ether modified silica resin.  CN102874889A
Ye  G., Bai F., Wei, J., et al. Palladium separation by  using double-armed cycloaliphatic crown ether modified silica resin.  CN102849823A
Ye  G., Wei J., Wang J., et al. Catalytic hydrogenation  synthesis of crown ether derivatives using the Pichler Ru catalyst, CN 102336737  A.
Ye  G., Wei J., Wang J., et al. Method for separation and  purification of crown ether stereoisomer, CN 102344435 A.
Ye  G., Bai F., Wei, J., et al. Preparation of a  cycloaliphatic crown ether modified silica resin.  CN102585231A.
Ye  G., Gao J., Wang J., et al. Process for preparation of  alkyl-substituted benzocrown ethers, CN 102167692 A.
Ye  G., He Y., Qu Z., et al. Fabrication of optical  waveguide using azobenzene-containing polymer. CN101762847A.

Last updated:2020-10-06